A Liquid Crystal Ionomer-Type Electrolyte toward Ordering-Induced Regulation for Highly Reversible Zinc Ion Battery

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成果类型：

期刊论文

作者：

Yuan, Du;Li, Xin;Yao, Hong;Li, Yuhang;Zhu, Xiaobo;...

通讯作者：

Yuan, Du(yuandu@csust.edu.cn);Zhao, Jin(iamjzhao@njupt.edu.cn);Zhang, Haitao(htzhang@ipe.ac.cn);Srinivasan, Madhavi(Madhavi@ntu.edu.sg)

作者机构：

[Yao, Hong; Yuan, Du; Li, Yuhang; Zhu, Xiaobo; Li, Xin] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410004, Hunan, Peoples R China.

[Zhao, Jin] Nanjing Univ Posts & Telecommun, State Key Lab Organ Elect & Informat Displays, 9 Wenyuan Rd, Nanjing 210023, Peoples R China.

[Zhao, Jin] Nanjing Univ Posts & Telecommun, Inst Adv Mat IAM, 9 Wenyuan Rd, Nanjing 210023, Peoples R China.

[Zhang, Haitao] Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China.

[Zhang, Yizhou] Nanjing Univ Informat Sci & Technol, Inst Adv Mat & Flexible Elect IAMFE, Sch Chem & Mat Sci, Nanjing 210044, Peoples R China.

通讯机构：

[Du Yuan; Du Yuan Du Yuan Du Yuan] C

[Jin Zhao; Madhavi Srinivasan; Jin Zhao Jin Zhao Jin Zhao; Madhavi Srinivasan Madhavi Srinivasan Madhavi Srinivasan] S

[Haitao Zhang; Haitao Zhang Haitao Zhang Haitao Zhang] I

Institute of Process Engineering, Chinese Academy of Sciences, Beijing, 100190 China<&wdkj&>College of Materials Science and Engineering, Changsha University of Science and Technology, Changsha, Hunan, 410004 P. R. China<&wdkj&>School of Materials Science and Engineering, Nanyang Technological University, Block N4.150 Nanyang Avenue, Singapore, 639798 Singapore<&wdkj&>State Key Laboratory of Organic Electronics and Information Displays & Institute of Advanced Materials (IAM), Nanjing University of Posts & Telecommunications, 9 Wenyuan Road, Nanjing, 210023 China

语种：

英文

关键词：

ionomer;liquid crystal electrolyte;ordering;zinc ion battery;Zn

期刊：

Advanced Science

ISSN：

2198-3844

年：

2023

卷：

期：

页码：

2206469-

DOI：

10.1002/advs.202206469

基金类别：

100 Talented Team of Hunan Province [XiangZu [2016] 91]; Natural Science Foundation of Hunan Province [2022JJ30613]; National Natural Science Foundation of China [21878308]; Natural Science Foundation of Jiangsu Province of China [BK20210604]; A*STAR under the Advanced Manufacturing and Engineering (AME) programmatic fund [A20H3g2140]; National Research Foundation of Singapore (NRF) Investigatorship Award [NRF-NRFI2017-08]

机构署名：

本校为第一机构

院系归属：

材料科学与工程学院

摘要：

Novel electrolyte is being pursued toward exploring Zn chemistry in zinc ion batteries. Here, a fluorine-free liquid crystal (LC) ionomer-type zinc electrolyte is presented, achieving simultaneous regulated water activity and long-range ordering of conduction channels and SEI. Distinct from water network or local ordering in current advances, long-range ordering of layered water channels is realized. Via manipulating water activity, conductivities range from ≈0.34 to 15 mS cm−1, and electrochemical window can be tuned from ≈2.3–4.3V. The Zn...

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A Liquid Crystal Ionomer-Type Electrolyte toward Ordering-Induced Regulation for Highly Reversible Zinc Ion Battery

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