Bi-affinity Electrolyte Optimizing High-Voltage Lithium-Rich Manganese Oxide Battery via Interface Modulation Strategy

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成果类型：

期刊论文

作者：

Yuan, Xuedi;Dong, Tao*;Liu, Jiaxin;Cui, Yingyue;Dong, Haotian;...

通讯作者：

Dong, Tao;Zhang, HT

作者机构：

[Dong, Tao; Liu, Jiaxin; Cui, Yingyue; Dong, Haotian; Zhang, Haitao; Yuan, Xuedi] Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China.

[Dong, Haotian; Zhang, Haitao; Yuan, Xuedi] Zhengzhou Univ, Sch Henan Inst Adv Technol, Zhengzhou 450002, Peoples R China.

[Zhang, Haitao] Zhengzhou Inst Emerging Ind Technol, Henan Key Lab Energy Storage Mat & Proc, Zhengzhou 450003, Peoples R China.

[Yuan, Du] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, 960,2 Sect, Changsha 410004, Hunan, Peoples R China.

通讯机构：

[Dong, T; Zhang, HT ] C

Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China.

Zhengzhou Inst Emerging Ind Technol, Henan Key Lab Energy Storage Mat & Proc, Zhengzhou 450003, Peoples R China.

语种：

英文

关键词：

Bi-Affinity Electrolyte;Ethyl Vinyl Sulfone;Fluoroethylene Carbonate;Interphase Modulation Strategy;Lithium Rich Manganese Oxide Cathode

期刊：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN：

1433-7851

年：

2023

卷：

期：

页码：

e202304121-

DOI：

10.1002/anie.202304121

基金类别：

National Key Research and Development Program of China [2022YFA1504103]; Science and Technology Service Network Initiative program of CAS [STS-QYZD-2021-02-002]; Joint Fund for Regional Innovation and Development [U22A20417]; ZhongKe-YuNeng Joint RD center [ZKYN2022006]; International Cooperative Project of CAS [122111KYSB20210012]

机构署名：

本校为其他机构

院系归属：

材料科学与工程学院

摘要：

The practical implementation of high‐voltage lithium‐rich manganese oxide (LRMO) cathode is limited by the formation of dendrites, unanticipated electrolyte decomposition, and dissolution of transition metal ions. The present study proposes a bi‐affinity electrolyte formulation, wherein the sulfonyl group of ethyl vinyl sulfone (EVS) imparts a highly adsorptive nature to LRMO, while fluoroethylene carbonate (FEC) exhibits a reductive nature towards Li metal. This interface modulation strategy involves the synergistic use of EVS and FEC as ad...

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Bi-affinity Electrolyte Optimizing High-Voltage Lithium-Rich Manganese Oxide Battery via Interface Modulation Strategy

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