Continuous Photocatalytic Acetylene Conversion to Ethylene in Liquid Under Ambient Conditions

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成果类型：

期刊论文

作者：

Lei, Xiaojia;Lei, Chao;Wang, Xuxu;Chen, Wenqian;Guo, Qian;...

通讯作者：

Huang, BB

作者机构：

[Lei, Xiaojia; Wang, Xuxu; Guo, Qian; Huang, Binbin] Hunan Univ, Coll Environm Sci & Engn, Key Lab Environm Biol & Pollut Control, Minist Educ, Changsha 410082, Peoples R China.

[Lei, Xiaojia; Huang, Binbin] Hunan Univ Chongqing, Res Inst, Chongqing 401100, Peoples R China.

[Lei, Chao] Changsha Univ Sci & Technol, Sch Hydraul Engn, Changsha 410114, Peoples R China.

[Chen, Wenqian] Natl Univ Singapore, Dept Pharm & Pharmaceut Sci, Sci Dr 4, Singapore 117560, Singapore.

[Hu, Yongyou] South China Univ Technol, Sch Environm & Energy, Guangzhou 510006, Peoples R China.

通讯机构：

[Huang, BB ] H

Hunan Univ, Coll Environm Sci & Engn, Key Lab Environm Biol & Pollut Control, Minist Educ, Changsha 410082, Peoples R China.

Hunan Univ Chongqing, Res Inst, Chongqing 401100, Peoples R China.

语种：

英文

关键词：

Atomic hydrogen;Ethylene purification and production;Photocatalytic acetylene hydrogenation;Photosynthesis;Proton coupled electron transfer

期刊：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN：

1433-7851

年：

2025

页码：

e202511422

DOI：

10.1002/anie.202511422

基金类别：

National Natural Science Foundation of China; Natural Science Foundation of Chongqing [CSTB2025jsyj-gkjzX0001]; Natural Science Foundation of Hunan Province [2023JJ30134]; [5177091149]

机构署名：

本校为其他机构

院系归属：

水利工程学院

摘要：

Ethylene is a basic building block for polymer synthesis, but its purification from petroleum-based processes (e.g., thermo-catalytic acetylene hydrogenation) and its production from coal-based processes (e.g., Fischer-Tropsch synthesis) normally require high temperature, high pressure, and gaseous hydrogen. Here, we report a continuous ethylene photosynthesis approach as a new platform technology that enables highly efficient and selective conversion of acetylene to ethylene in liquid under mild conditions. This platform technology is compatible with a wide range of solvents, catalysts, and h...

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Continuous Photocatalytic Acetylene Conversion to Ethylene in Liquid Under Ambient Conditions

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