The bond between carbon fiber-reinforced polymer (CFRP) composites and steel is a key issue in CFRP-strengthened steel structures. The determination of key parameters in the bond strength model remains debatable. We studied the bond behavior between CFRP and steel, focusing on the effects of different types of epoxy adhesive and CFRP on the failure modes, bond–slip relationships, and bond strength parameters. The results show that due to the use of various materials, some specimens fail in interface debonding characterized by brittle failure, ...