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In situ synthesis of Ni-based catalyst for ambient-temperature CO2 methanation using rare-metal hydrides: Unveiling the reaction pathway and catalytic mechanism

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成果类型:
期刊论文
作者:
Kang Chen;Yunqi Jia;Fen Liu;Xusheng Yang;Yi Jia;...
通讯作者:
Xusheng Yang<&wdkj&>Yi Jia<&wdkj&>Liuzhang Ouyang
作者机构:
[Yunqi Jia; Fen Liu; Jiangwen Liu; Hui Wang] School of Materials Science and Engineering, Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials, South China University of Technology, Guangzhou 510641, China
Key Laboratory of Energy Efficient & Clean Utilization, School of Energy and Power Engineering, Changsha University of Science and Technology, Changsha 410114, China
[Xusheng Yang] Department of Industrial and Systems Engineering, Research Institute for Advanced Manufacturing, the Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong, China
China-Australia Joint Laboratory for Energy & Environmental Materials, Key Laboratory of Fuel Cell Technology of Guangdong Province, Guangzhou 510641, China
School of Natural Sciences and Queensland Micro- and Nanotechnology Centre, Griffith University, Nathan, QLD 4111, Australia
通讯机构:
[Xusheng Yang] D
[Yi Jia] C
[Liuzhang Ouyang] S
Department of Industrial and Systems Engineering, Research Institute for Advanced Manufacturing, the Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong, China<&wdkj&>China-Australia Joint Laboratory for Energy & Environmental Materials, Key Laboratory of Fuel Cell Technology of Guangdong Province, Guangzhou 510641, China<&wdkj&>School of Natural Sciences and Queensland Micro- and Nanotechnology Centre, Griffith University, Nathan, QLD 4111, Australia<&wdkj&>School of Materials Science and Engineering, Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials, South China University of Technology, Guangzhou 510641, China<&wdkj&>China-Australia Joint Laboratory for Energy & Environmental Materials, Key Laboratory of Fuel Cell Technology of Guangdong Province, Guangzhou 510641, China
语种:
英文
期刊:
材料科学技术(英文)
ISSN:
1005-0302
年:
2026
卷:
242
页码:
92-101
基金类别:
CRediT authorship contribution statement Kang Chen: Writing – original draft, Methodology, Investigation, acquisition, Formal analysis, Data curation, Conceptualization. Yunqi Jia: Writing – original draft, Validation, Investigation, Data curation. Fen Liu: Investigation, Formal analysis, Data curation. Xusheng Yang: Writing – review & editing, Validation, acquisition. Yi Jia: Validation, Supervision, Methodology, Formal analysis. Jiangwen Liu: Validation, Formal analysis. Hui Wang: Validation, Formal analysis.
机构署名:
本校为其他机构
院系归属:
能源与动力工程学院
摘要:
Converting CO 2 into high value-added chemical fuels through coupling with renewable hydrogen, has emerged as a pivotal strategy to address environmental pollution and tackle energy supply issues. However, the high chemical inertness of CO 2 molecules and the complex multi-electron transfer processes involved in CO 2 hydrogenation pose significant challenges, leading to large energy barriers and poor product selectivity. Traditional chemical catalysts typically require harsh conditions such as high temperatures, pressures, and/or additives to overcome these barriers and accelerate sluggish rea...

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