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Semi-closed synthesis of nitrogen and oxygen Co-doped mesoporous carbon for selective aqueous oxidation

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成果类型:
期刊论文
作者:
Xing, Chen;Yang, Daihui;Zhang, Yan*;Sun, Tian;Duan, Junfei;...
通讯作者:
Zhang, Yan;Zhang, Shiguo
作者机构:
[Sun, Tian; Xing, Chen; Zhang, Y; Zhang, Shiguo; Yang, Daihui; Zhang, Yan; Younus, Hussein A.] Hunan Univ, Coll Mat Sci & Engn, Hunan Prov Key Lab Adv Carbon Mat & Appl Technol, Changsha 410082, Hunan, Peoples R China.
[Duan, Junfei] Changsha Univ Sci & Technol, Sch Mat Sci & Engn, Changsha 410004, Peoples R China.
[Younus, Hussein A.] Fayoum Univ, Fac Sci, Chem Dept, Al Fayyum 63514, Egypt.
通讯机构:
[Zhang, Y; Zhang, SG] H
Hunan Univ, Coll Mat Sci & Engn, Hunan Prov Key Lab Adv Carbon Mat & Appl Technol, Changsha 410082, Hunan, Peoples R China.
语种:
英文
关键词:
Semi-closed carbonization;Nitrogen and oxygen doping;Mesoporous carbon;Metal-free catalyst;Selective aqueous oxidation
期刊:
绿色能源与环境(英文)
ISSN:
2096-2797
年:
2022
卷:
7
期:
1
页码:
43-52
基金类别:
supported by National Natural Science Foundation of China (Grant No. 51772089 and 21872046); the Youth 1000 Talent Program of China; the Outstanding Youth Scientist Foundation of Hunan Province (Grant No. 2018JJ1009); the Natural Science Foundation of Hunan Province (Grant No. 2020JJ4174); Provincial Science and Technology Innovation Platform and Talent Plan-Changsha, Zhuzhou and Xiangtan High-level Talents Accumulation Project (Grant No. 2017XK2023); Research and Development Plan of Key Areas in Hunan Province (Grant No. 2019GK2235);
机构署名:
本校为其他机构
院系归属:
材料科学与工程学院
摘要:
Heteroatom-doped meso/micro-porous carbon materials are conventionally produced by harsh carbonization under an inert atmosphere involving specific precursors, hard/soft templates, and heteroatom-containing agents. Herein, we report a facile synthesis of N and O co-doped meso/micro-porous carbon (NOMC) by template-free carbonization of a small-molecule precursor in a semi-closed system. The semi-closed carbonizaiton process yields hydrophilic NOMCs with large surface area in a high yield. The porous structure as well as the elemental compositio...

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