High performance and long cycle life neutral zinc-iron flow batteries enabled by zinc-bromide complexation

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成果类型：

期刊论文

作者：

Yang, Minghui;Xu, Zhizhao;Xiang, Weizhe;Xu, He;Ding, Mei*;...

通讯作者：

Ding, Mei;Jia, Chuankun;Tang, Ao;Zhou, Guangmin

作者机构：

[Yang, Minghui; Xu, He; Xu, Zhizhao; Li, Liangyu; Jia, Chuankun; Ding, Mei; Jia, CK; Xiang, Weizhe] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Peoples R China.

[Jia, Chuankun; Ding, Mei] Changsha Univ Sci & Technol, Sch Traff & Transportat Engn, Natl Engn Lab Highway Maintenance Technol, Changsha 410114, Peoples R China.

[Tang, Ao] Chinese Acad Sci, Inst Met Res, Shenyang 110016, Peoples R China.

[Zhou, Guangmin; Gao, Runhua] Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen Geim Graphene Ctr, Shenzhen 518055, Peoples R China.

[Zhou, Guangmin; Gao, Runhua] Tsinghua Univ, Tsinghua Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China.

通讯机构：

[Ding, M; Jia, CK; Tang, Ao] C

[Zhou, Guangmin] T

Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Peoples R China.

Chinese Acad Sci, Inst Met Res, Shenyang 110016, Peoples R China.

Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen Geim Graphene Ctr, Shenzhen 518055, Peoples R China.

语种：

英文

关键词：

Complexation interaction;Electrochemical energy storage;Electrolyte additive;Redox reversibility;Zn/Fe flow batteries

期刊：

Energy Storage Materials

ISSN：

2405-8297

年：

2022

卷：

页码：

433-440

DOI：

10.1016/j.ensm.2021.10.043

基金类别：

The authors acknowledge the financial supports from the 100 Talented Team of Hunan Province (Xiang Zu [2016] 91), the “Huxiang High-level talents” programs (No. 2018RS3077 and 2019RS1046), the Natural Science Foundation of Hunan Province (2020JJ5566) and the Open Fund of National Engineering Laboratory of Highway Maintenance Technology (Changsha Univeristy of Science & Technology) (No. kjf170105). G. Z. appreciates the support from the National Key Research and Development Program of China (2019YFA0705700), National Natural Science Foundation of China (No. 52072205) and Shenzhen Geim Graphene Center.

机构署名：

本校为第一且通讯机构

院系归属：

交通运输工程学院

材料科学与工程学院

摘要：

Zinc-based flow batteries have attracted tremendous attention owing to their outstanding advantages of high theoretical gravimetric capacity, low electrochemical potential, rich abundance, and low cost of metallic zinc. Among which, zinc-iron (Zn/Fe) flow batteries show great promise for grid-scale energy storage. However, they still face challenges associated with the corrosive and environmental pollution of acid and alkaline electrolytes, hydrolysis reactions of iron species, poor reversibility and stability of Zn/Zn2+ redox couple. In this w...

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High performance and long cycle life neutral zinc-iron flow batteries enabled by zinc-bromide complexation

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