Redox Targeting-based Neutral Aqueous Flow Battery with High Energy Density and Low Cost

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成果类型：

期刊论文

作者：

Yan, Su;Huang, Songpeng;Xu, He;Li, Liangyu;Zou, Haitao;...

通讯作者：

Ding, Mei;Jia, CK;Wang, Q

作者机构：

[Zou, Haitao; Xu, He; Li, Liangyu; Jia, Chuankun; Ding, Mei; Yan, Su] Changsha Univ Sci & Technol, Inst Energy Storage Technol, Changsha 410114, Peoples R China.

[Xu, He; Li, Liangyu; Jia, Chuankun; Ding, Mei; Yan, Su] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Peoples R China.

[Huang, Songpeng; Wang, Qing] Natl Univ Singapore, Coll Design & Engn, Dept Mat Sci & Engn, Singapore 117576, Singapore.

[Wang, Qing] Natl Univ Singapore, Coll Design & Engn, Dept Mat Sci & Engn, Singapore 117576, Singapore.

[Jia, CK; Ding, Mei] Changsha Univ Sci & Technol, Inst Energy Storage Technol, Changsha 410114, Peoples R China.

通讯机构：

[Wang, Q ; Jia, CK ; Ding, M]

Changsha Univ Sci & Technol, Inst Energy Storage Technol, Changsha 410114, Peoples R China.

Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Peoples R China.

Natl Univ Singapore, Coll Design & Engn, Dept Mat Sci & Engn, Singapore 117576, Singapore.

语种：

英文

关键词：

redox mediator;flow batteries;redox-targeting reaction;Prussian blue;polysulfides

期刊：

ChemSusChem

ISSN：

1864-5631

年：

2023

卷：

期：

页码：

e202300710-

DOI：

10.1002/cssc.202300710

基金类别：

National Key Research and Development Program of China [2022YFB2405100]; National Natural Science Foundation of China [22209015]; Scientific Research Foundation of Hunan Provincial Education Department [21A0195]; 100 Talented Team of Hunan Province [[2016] 91]

机构署名：

本校为第一且通讯机构

院系归属：

材料科学与工程学院

摘要：

A neutral aqueous single‐molecule redox‐targeting (SMRT)‐based Prussian blue (PB)−Fe/S flow battery was demonstrated. Especially, the energy density of a battery based on [Fe(CN)6]3−/4−‐containing catholyte is increased to 92.8 Wh L−1. Moreover, the PB−Fe/S flow battery exhibits outstanding performance with long cycle life over 7000 cycles (4500 h), and the chemical cost of the PB−Fe/S full cell is as low as 19.26 $ kWh−1. Abstract Neutral aqueous flow batteries with common traits of the redox flow batteries, such as the indepe...

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Redox Targeting-based Neutral Aqueous Flow Battery with High Energy Density and Low Cost

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