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General and Ultrafast Photothermal Synthesis of Atomic Metal-Nitrogen-Carbon Catalysts for H2O2 Electrosynthesis

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成果类型:
期刊论文
作者:
Gong, Haisheng;Gong, Zhichao;Liu, Jingjing;Ye, Gonglan*;Fei, Huilong
通讯作者:
Ye, Gonglan;Fei, HL
作者机构:
[Gong, Haisheng; Ye, Gonglan; Fei, Huilong; Gong, Zhichao] Hunan Univ, Adv Catalyt Engn Res Ctr, State Key Lab Chemo Biosensing & Chemometr, Minist Educ, Changsha 410082, Peoples R China.
[Gong, Haisheng; Ye, Gonglan; Fei, Huilong; Gong, Zhichao] Hunan Univ, Coll Chem & Chem Engn, Changsha 410082, Peoples R China.
[Liu, Jingjing] Changsha Univ Sci & Technol, Sch Mat Sci & Engn, Changsha 410114, Peoples R China.
通讯机构:
[Ye, GL; Fei, HL ] H
Hunan Univ, Adv Catalyt Engn Res Ctr, State Key Lab Chemo Biosensing & Chemometr, Minist Educ, Changsha 410082, Peoples R China.
Hunan Univ, Coll Chem & Chem Engn, Changsha 410082, Peoples R China.
语种:
英文
关键词:
flash light irradiation;generality;H2O2 electrosynthesis;photothermal synthesis;single-atom catalysts
期刊:
Advanced Functional Materials
ISSN:
1616-301X
年:
2024
基金类别:
National Natural Science Foundation of China; Major Program of the Natural Science Foundation of Hunan Province [2021JC0006]; [22209043]
机构署名:
本校为其他机构
院系归属:
材料科学与工程学院
摘要:
Atomic metal-nitrogen-carbon catalysts (M-N-Cs) are promising electrocatalysts for the two-electron oxygen reduction reaction (2e(-) ORR) for the green production of H2O2. However, the conventional synthetic methods of M-N-Cs typically suffer from prolonged possessing time and high energy consumption. Herein, a flash light irradiation-assisted transient pyrolysis strategy is reported for the rapid and facile synthesis of a Co-N-C catalyst consisting of atomic Co-N-4 sites supported on graphene. The resultant Co-N-C is highly active and selective as an electrocatalyst for the 2e(-) ORR, with a ...

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