Plastic Deformation of LiNi0.5Mn1.5O4 Single Crystals Caused by Domain Orientation Dynamics

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作者信息关键词期刊信息基础信息归属信息摘要

成果类型：

期刊论文

作者：

Vostrov, Nikita;Martens, Isaac;Colalongo, Mattia;Zatterin, Edoardo;Ronovsky, Michal;...

通讯作者：

Richard, Marie-Ingrid;Schulli, T;Richard, MI

作者机构：

[Richard, Marie-Ingrid; Schulli, T; Zatterin, Edoardo; Richard, MI; Schulli, Tobias; Leake, Steven; Colalongo, Mattia; Martens, Isaac; Vostrov, Nikita] ESRF The European Synchrotron, 71 Ave Martyrs, Grenoble, France.

[Ronovsky, Michal] Univ Grenoble Alpes, CNRS, Grenoble INP, LEPMI, F-38402 St Martin Dheres, France.

[Boulineau, Adrien] Univ Grenoble Alpes, CEA Liten, F-38000 Grenoble, France.

[Zhu, Xiaobo] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Peoples R China.

[Wang, Lianzhou] Univ Queensland, Nanomat Ctr, Sch Chem Engn, St Lucia, Qld 4072, Australia.

通讯机构：

[Schulli, T ; Richard, MI] E

[Richard, MI ] U

ESRF The European Synchrotron, 71 Ave Martyrs, Grenoble, France.

Univ Grenoble Alpes, CEA Grenoble, IRIG, MEM,NRX, 17 Rue Martyrs, F-38000 Grenoble, France.

语种：

英文

关键词：

high voltage cathode;Li-ion batteries;LMNO;spinel;SXDM

期刊：

Advanced Energy Materials

ISSN：

1614-6832

年：

2025

卷：

期：

页码：

2404933

DOI：

10.1002/aenm.202404933

基金类别：

HORIZON EUROPE European Research Council [814106, 818823]; European Research Council (ERC) under the European Union

机构署名：

本校为其他机构

院系归属：

材料科学与工程学院

摘要：

AbstractThe nanoscale mechanisms of ion deintercalation in battery cathode materials remain poorly understood, especially the relationship between crystallographic defects (dislocations, small angle grain boundaries, vacancies, etc), device performance, and durability. In this work, operando scanning X‐ray diffraction microscopy (SXDM) and multi‐crystal X‐ray diffraction (MCXD) are used to investigate microstrain and lattice tilt inhomogeneities inside Li1 − x Ni0.5Mn1.5O4 cathode particles during electrochemical cycling and their influence...

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Plastic Deformation of LiNi0.5Mn1.5O4 Single Crystals Caused by Domain Orientation Dynamics

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