Permanganate-promoted photocatalytic oxidation for efficient water treatment via a synergy of nonradical and radical relay process

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成果类型：

期刊论文

作者：

Wang, Xuxu;Yan, Sitong;Yang, Zilei;Chen, Wenqian;Lei, Xiaojia;...

通讯作者：

Huang, BB

作者机构：

[Huang, Binbin; Lei, Xiaojia; Yang, Zilei; Wang, Xuxu; Guo, Qian; Yan, Sitong] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Peoples R China.

[Wang, Xuxu] Univ Sci & Technol China, Dept Environm Sci & Technol, Hefei 230026, Peoples R China.

[Chen, Wenqian] Natl Univ Singapore, Dept Pharm, 4 Sci Dr 2, Singapore 117544, Singapore.

[Lei, Chao] Changsha Univ Sci & Technol, Sch Hydraul Engn, Key Lab Dongting Lake Aquat Ecoenvironm Control &, Changsha 410114, Peoples R China.

[Hu, Yongyou; Feng, Chunhua; Huang, Binbin] South China Univ Technol, Sch Environm & Energy, Key Lab Pollut Control & Ecol Remediat Ind Cluster, Minist Educ, Guangzhou 510006, Guangdong, Peoples R China.

通讯机构：

[Huang, BB ] H

Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Peoples R China.

语种：

英文

关键词：

Advanced oxidation processes (AOPs);Photocatalysis;Permanganate activation;Reactive manganese species;Radical

期刊：

Applied Catalysis B: Environmental

ISSN：

0926-3373

年：

2025

卷：

365

页码：

124993

DOI：

10.1016/j.apcatb.2024.124993

基金类别：

National Natural Science Founda-tion of China [5177091149]; China Postdoctoral Science Foundation [2024M763164]; Natural Science Foundation of Hunan Prov-ince and Changsha [2023JJ30134, kq2208034]; Na-tional Training Program of Innovation and Entrepreneurship for Undergraduates [S202310532494]

机构署名：

本校为其他机构

院系归属：

水利工程学院

摘要：

Radical- and nonradical-based advanced oxidation processes (AOPs) have been widely used as water cleaning technologies. It is a great challenge to achieve a synergy between these two methodologies for enhancing the performance of water purification. Here we report a novel strategy of permanganate (PM)-promoted photocatalytic oxidation by using TiO 2 with different ratios of (101) and (001) facets as model photocatalysts to achieve a synergy of nonradical-radical relay oxidation process. This approach can simultaneously trigger PM activation by photogenerated electrons and result in the selecti...

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Permanganate-promoted photocatalytic oxidation for efficient water treatment via a synergy of nonradical and radical relay process

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