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Post-Modification of MOF with Electron Donor for Efficient Photocatalytic Oxidative Organic Transformations

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成果类型:
期刊论文
作者:
Hong-Guang Jin*;Wei Lin;Huapeng Sun;Peng-Cheng Zhao;Jie Deng
通讯作者:
Hong-Guang Jin
作者机构:
[Hong-Guang Jin] Changsha University of Science and Technology, School of Materials Science and Engineering, Wanjiali Road, CHINA
[Huapeng Sun] Chenzhou Vocational Technical College, School of New Energy, CHINA
[Wei Lin; Peng-Cheng Zhao; Jie Deng] Changsha University of Science and Technology - Yuntang Campus: Changsha University of Science and Technology, School of Materials Science and Engineering, CHINA
通讯机构:
[Hong-Guang Jin] C
Changsha University of Science and Technology, School of Materials Science and Engineering, Wanjiali Road, CHINA
语种:
英文
关键词:
metal-organic framework;Organic transformation;Charge transfer;superoxide radical
期刊:
CHEMISTRY-A EUROPEAN JOURNAL
ISSN:
0947-6539
年:
2025
页码:
e202500015
机构署名:
本校为第一且通讯机构
院系归属:
材料科学与工程学院
摘要:
Construction of donor-accepter systems via self-assembling electron donor and acceptor chromophores within one single metal-organic framework (MOF) for advanced artificial photosynthesis is of great intertest yet a major challenge. Herein, an electron donor porphyrin 5-(4-carboxyphenyl)-10,15,20-triphenylporphyrin (PCOOH) was successfully integrated into a highly stable and porous electron acceptor naphthalene diimide (NDI)-based MOF (Zr-NDI) through the post-modified approach of solvent-assisted ligand incorporation (SALI). Benefiting from the...

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