Cu@Co with Dilatation Strain for High‐Performance Electrocatalytic Reduction of Low‐Concentration Nitric Oxide

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成果类型：

期刊论文

作者：

Wu, Ze;Liu, Yujing;Wang, Dongdong;Zhang, Yiqiong;Gu, Kaizhi;...

通讯作者：

Zhang, YQ;Wang, SY

作者机构：

[Fan, Jincheng; Wu, Ze; Liu, Yujing; Zhang, Yiqiong] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Hunan, Peoples R China.

[Wang, Dongdong; Wang, SY; Wang, Shuangyin; Chen, Chen] Hunan Univ, Coll Chem & Chem Engn, Natl Supercomp Ctr Changsha, State Key Lab Chem Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.

[Gu, Kaizhi] Cent South Univ, Inst Adv Study, Changsha 410083, Peoples R China.

[Liu, Hanwen] Curtin Univ, WA Sch Mines Minerals Energy & Chem Engn WASM MECE, Perth, WA 6102, Australia.

[He, Zejin; Liu, Limin] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China.

通讯机构：

[Wang, SY ] H

[Zhang, YQ ] C

Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Hunan, Peoples R China.

Hunan Univ, Coll Chem & Chem Engn, Natl Supercomp Ctr Changsha, State Key Lab Chem Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.

语种：

英文

关键词：

Cu@Co catalyst;NH3 synthesis;NO reduction;dilatation strain;electrocatalysis

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2024

卷：

期：

页码：

e2309470

DOI：

10.1002/adma.202309470

基金类别：

National Natural Science Foundation of China; Natural Science Foundation of Hunan Province [2023JJ20037, 2021JJ40565]; Postgraduate Scientific Research Innovation Project of Hunan Province [CX20230941]; [22372012]; [22261160640]; [22002009]; [22002039]

机构署名：

本校为第一且通讯机构

院系归属：

材料科学与工程学院

摘要：

In this work, a Cu@Co catalyst with dilatation strain is prepared for low‐concentration NO electroreduction, and it exhibits high NH3 yield of 627.20 µg h‐1 cm‐2 and Faradaic efficiency of 76.54%. The assembled Zn‐NO battery using Cu@Co as cathode achieves a power density of 3.08 mW cm−2, which can simultaneously realize NO removal, NH3 green synthesis, and electricity output. Abstract Electrocatalytic reduction of nitric oxide (NO) to ammonia (NH3) is a clean and sustainable strategy to simultaneously remove NO and synthesize NH3. Howeve...

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Cu@Co with Dilatation Strain for High‐Performance Electrocatalytic Reduction of Low‐Concentration Nitric Oxide

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