Electro-responsive Tri-state Switch in Supramolecular Circuits

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期刊论文

作者：

Tan, Min;Zhao, Xueyan;Zhao, Zhibin;Adijiang, Adila;Shu, Haibo;...

通讯作者：

Chen, Lichuan;Xiang, D;Fan, ZQ

作者机构：

[Tan, Min; Shu, Haibo] China Jiliang Univ, Coll Opt & Elect Technol, Hangzhou 310018, Peoples R China.

[Adijiang, Adila; Xiang, Dong; Zhao, Zhibin; Zhao, Xueyan; Chen, Lichuan; Tan, Min] Nankai Univ, Inst Modern Opt, Tianjin 300350, Peoples R China.

[Adijiang, Adila; Xiang, Dong; Zhao, Zhibin; Zhao, Xueyan; Chen, Lichuan; Tan, Min] Nankai Univ, Ctr Single Mol Sci, Tianjin Key Lab Microscale Opt Informat Sci & Tech, Tianjin 300350, Peoples R China.

[Zhao, Xueyan] Northeast Petr Univ, Sch Phys & Elect Engn, Daqing 163318, Peoples R China.

[Zhao, Zhibin] Henan Acad Sci, Inst Phys, Henan Engn Res Ctr Photoelect Measurement, Zhengzhou 450046, Peoples R China.

通讯机构：

[Xiang, D ; Chen, LC] N

[Fan, ZQ ] C

Nankai Univ, Inst Modern Opt, Tianjin 300350, Peoples R China.

Nankai Univ, Ctr Single Mol Sci, Tianjin Key Lab Microscale Opt Informat Sci & Tech, Tianjin 300350, Peoples R China.

Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha 410114, Peoples R China.

语种：

英文

关键词：

Charge transport;Molecular electronics;Molecular switch;Supramolecular junction

期刊：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN：

1433-7851

年：

2025

卷：

期：

页码：

e202511115

DOI：

10.1002/anie.202511115

基金类别：

National Key R&D Program of China; National Natural Science Foundation of China [22273041, 12174201]; Natural Science Foundation of Tianjin [19JCZDJC31000, 19JCJQJC60900, 22JCYBJC01310]; [2021YFA1200103]

机构署名：

本校为通讯机构

院系归属：

物理与电子科学学院

摘要：

Efficiently manipulating charge transport at the molecular level is critical to developing multifunctional and responsive molecular electronic devices. Here, we report the first electroresponsive tristate switch in a supramolecular circuit, overcoming the binary limitation and enabling richer logic encoding, governed solely by a bias voltage (electric field). At low electric fields, p-phenylenediamine (PPD) molecules exhibit a high-conductance state, which transitions successively to two distinct low-conductance states as the external electric ...

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Electro-responsive Tri-state Switch in Supramolecular Circuits

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