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Thermal conduction-induced crystallization and achieving high efficiency in HTM-free carbon-based CsPbI2Br solar cells by regulating the dipole moment of aliphatic amine acetate additives

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成果类型:
期刊论文
作者:
Zhang, Xinlong;Huang, Jincheng*;Zuo, Hengzhi;Zhang, Yuanfang;Guo, Yuhang;...
通讯作者:
Huang, Jincheng;Peng, ZY
作者机构:
[Huang, Jincheng; Zhang, Yuanfang; Peng, Zhuoyin; Guo, Yuhang; Zhang, Xinlong; Li, Wei; Peng, ZY; Zuo, Hengzhi; Chen, Jianlin] Changsha Univ Sci & Technol, Sch Energy & Power Engn, Key Lab Efficient & Clean Energy Utilizat, Changsha 410111, Peoples R China.
[Shi, Yifei] Changsha Univ Sci & Technol, Sch Elect & Informat Engn, Changsha 410114, Peoples R China.
[Li, Guijun] Shenzhen Univ, Key Lab Optoelect Devices & Syst, Minist Educ, Shenzhen 518060, Peoples R China.
[Li, Guijun] Shenzhen Univ, Coll Phys & Optoelect Engn, Shenzhen 518060, Guangdong, Peoples R China.
通讯机构:
[Huang, JC; Peng, ZY ] C
Changsha Univ Sci & Technol, Sch Energy & Power Engn, Key Lab Efficient & Clean Energy Utilizat, Changsha 410111, Peoples R China.
语种:
英文
期刊:
Journal of Materials Chemistry C
ISSN:
2050-7526
年:
2025
基金类别:
National Natural Science Foundation of China [52172183]; Natural Science Foundation of Hunan Province, China [2024JJ5025, 2022JJ40513]; Outstanding Youth Scientific Research Project of the Education Department of Hunan Province [21B0316, 22C0161]; Chunhui Plan" Cooperative Scientific Research Project of Chinese Ministry of Education [HZKY20220361]; Changsha Natural Science Foundation [kq2208220]; Scientists Sponsorship Program by Hunan Province [2023TJ-Z30]; Postgraduate Scientific Research Innovation Project of Hunan Province [QL20230215]
机构署名:
本校为第一且通讯机构
院系归属:
电气与信息工程学院
能源与动力工程学院
摘要:
Despite the advancements in film fabrication techniques for emerging perovskite solar cells, achieving a high-quality film by solution processing, while maintaining considerable performance remains a significant challenge. To tackle the issue of inferior CsPbI2Br perovskite films deposited via solution-based methods, a novel thermal conduction heating approach was devised and implemented, significantly enhancing film uniformity. Crucially, aliphatic amine acetates (3A) were introduced into the precursor solution to regulate the crystallization process and therefore to mitigate defects. Systema...

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