Reconstruction of Ultrahigh-Aspect-Ratio Crystalline Bismuth–Organic Hybrid Nanobelts for Selective Electrocatalytic CO2 Reduction to Formate

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成果类型：

期刊论文

作者：

Zeng, Guang;He, Yingchun;Ma, Dong-Dong;Luo, Shiwen;Zhou, Shenghua;...

通讯作者：

Zhu, QL

作者机构：

[Ma, Dong-Dong; Wu, Xin-Tao; Zeng, Guang; Cao, Changsheng; Li, Xiaofang; He, Yingchun; Zhu, Qi-Long; Zhou, Shenghua] Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Peoples R China.

[Zeng, Guang] Changsha Univ Sci & Technol, Sch Mat Sci & Engn, Changsha 410004, Peoples R China.

[He, Yingchun; Zhu, Qi-Long; Zhou, Shenghua] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.

[Liao, Hong-Gang; Luo, Shiwen] Xiamen Univ, State Key Lab Phys Chem Solid Surfaces, Coll Chem & Chem Engn, Xiamen 361005, Peoples R China.

[Wu, Xin-Tao; Zhu, Qi-Long] Fujian Sci & Technol Innovat Lab Optoelect Inform, Fuzhou 350108, Peoples R China.

通讯机构：

[Zhu, QL ] C

Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Peoples R China.

Univ Chinese Acad Sci, Beijing 100049, Peoples R China.

Fujian Sci & Technol Innovat Lab Optoelect Inform, Fuzhou 350108, Peoples R China.

语种：

英文

关键词：

bismuth;CO 2 reduction reactions;edge sites;electrocatalysis;formate;nanobelts

期刊：

Advanced Functional Materials

ISSN：

1616-301X

年：

2022

卷：

期：

页码：

2201125-

DOI：

10.1002/adfm.202201125

基金类别：

G.Z. and Y.H. contributed equally to this work. The authors are grateful for the financial support of the National Key Research and Development Program of China (2021YFA1500402), the National Natural Science Foundation of China (NSFC) (21905278, 22105203, and 22175174), the Natural Science Foundation of Fujian Province (2019J05158, 2020J01116 and 2021J06033), and the China Postdoctoral Science Foundation (2021TQ0332 and 2021M703215).

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本校为其他机构

院系归属：

材料科学与工程学院

摘要：

The morphology and active site engineering of electrocatalysts is an efficient strategy to improve the intrinsic activity and selectivity of electrocatalytic CO2 reduction. Here the ultralong and thin Bi nanobelts (Bi-NBs) are fabricated, which feature a high edge-to-facet ratio and high-degree connectivity is inherited from the ultrahigh-aspect-ratio crystalline bismuth−organic hybrid nanobelts, through a cathodically in situ reconstruction process. The unique nanostructure of Bi-NBs leads to a significantly enhanced performance for electroca...

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Reconstruction of Ultrahigh-Aspect-Ratio Crystalline Bismuth–Organic Hybrid Nanobelts for Selective Electrocatalytic CO2 Reduction to Formate

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