A strong nucleophilic fluorination agent to achieve highly stable in-situ 3D cross-linked gel polymer electrolyte for lithium-ion batteries

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成果类型：

期刊论文

作者：

Zhang, Libo;Bai, Maohui*;Wang, Xuhui;Huang, Zimo;Hong, Bo;...

通讯作者：

Bai, Maohui;Hong, B;Huang, ZM

作者机构：

[Zhang, Libo; Bai, Maohui; Hong, Bo; Lai, Yanqing] Cent South Univ, Sch Met & Environm, Changsha 410083, Peoples R China.

[Wang, Xuhui; Bai, Maohui] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410004, Peoples R China.

[Huang, ZM; Huang, Zimo] Guangdong Univ Technol, Sch Chem Engn & Light Ind, Inst Sustainable Transformat, Guangzhou 510006, Peoples R China.

[Zhang, Libo; Hong, Bo; Lai, Yanqing] Cent South Univ, Hunan Prov Key Lab Nonferrous Value Added Met, Changsha 410083, Peoples R China.

通讯机构：

[Huang, ZM ] G

[Bai, MH; Hong, B ] C

Cent South Univ, Sch Met & Environm, Changsha 410083, Peoples R China.

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Inst Sustainable Transformat, Guangzhou 510006, Peoples R China.

语种：

英文

关键词：

Nucleophilic fluorination;Li metal anode;In-situ polymerization;Gel polymer electrolyte

期刊：

Chemical Engineering Journal

ISSN：

1385-8947

年：

2024

卷：

481

页码：

148579

DOI：

10.1016/j.cej.2024.148579

基金类别：

CRediT authorship contribution statement Libo Zhang: Writing – original draft, Investigation, Data curation. Maohui Bai: Writing – review & editing, Supervision, Project administration, acquisition. Xuhui Wang: Formal analysis. Zimo Huang: Supervision, Methodology. Bo Hong: Writing – review & editing, Supervision, Conceptualization. Yanqing Lai: Supervision, Project administration, acquisition.

机构署名：

本校为其他机构

院系归属：

材料科学与工程学院

摘要：

The Gel Polymer Electrolyte (GPE) is recognized as a promising alternative to conventional electrolytes, aiming to enhance the longevity and energy density of lithium-ion batteries (LIBs). However, several challenges persist, particularly concerning the conductivity and voltage window of GPE in battery systems. In this study, we introduce an in-situ 3D crosslinked GPE, using polymethyl methacrylate (PMMA) as the monomer and polyethylene glycol dimethacrylate (PEGDMA) as the crosslinking agent, to ensure structural stability and optimized ion conductivity. We also incorporate a potent nucleophi...

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A strong nucleophilic fluorination agent to achieve highly stable in-situ 3D cross-linked gel polymer electrolyte for lithium-ion batteries

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