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Activation of sodium percarbonate by micro amounts of copper for highly efficient degradation of acid orange 7

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成果类型:
期刊论文
作者:
Liu, Yuanyuan;Xia, Yan;Xiong, Ying;Zhang, Shuhao;Yu, Jian;...
通讯作者:
Xiong, Y;Wang, JJ
作者机构:
[Xiong, Ying; Liu, Yuanyuan] Changsha Univ Sci & Technol, Res Ctr Resource Environm & Urban Planning, Sch Architecture, Changsha 410114, Hunan, Peoples R China.
[Tang, Xianghui; Lin, Ziwei; Xia, Yan; Deng, Yuwei; Wu, Haipeng; Xiong, Ying] Changsha Univ Sci & Technol, Sch Hydraul & Environm Engn, Changsha 410114, Hunan, Peoples R China.
[Yu, Jian; Zhang, Shuhao] China Railway Dev Investment Grp Co Ltd, Kunming 650100, Yunnan, Peoples R China.
[Wang, Jiajia] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China.
通讯机构:
[Xiong, Y ] C
[Wang, JJ ] H
Changsha Univ Sci & Technol, Res Ctr Resource Environm & Urban Planning, Sch Architecture, Changsha 410114, Hunan, Peoples R China.
Changsha Univ Sci & Technol, Sch Hydraul & Environm Engn, Changsha 410114, Hunan, Peoples R China.
Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China.
语种:
英文
关键词:
Micro -amount cupric species;Sodium percarbonate;Advanced oxidation processes;Reactive oxygen species;Cu(III)
期刊:
Separation and Purification Technology
ISSN:
1383-5866
年:
2023
卷:
322
页码:
124256
基金类别:
The decomposition of AO7 under various conditions are demonstrated in Fig. 1a. Cu(II) or SPC alone could barely degrade AO7, indicating weak capability to decompose AO7 by Cu(II) or SPC, consistent with the previous results reported [20]. Remarkably, the co-presence of Cu(II) and SPC in the system resulted in relatively fast decolorization of AO7, with approximately 90% of AO7 degraded in the first 2 min, and around 95% of AO7 was removed within 15 min, suggesting the triggering effects of SPC
机构署名:
本校为第一且通讯机构
院系归属:
建筑学院
摘要:
In recent years, activation of sodium percarbonate (SPC) has been regarded as very appealing technologies in the elimination of organic pollutants. In this work, the activation of SPC using micro amounts of Cu(II) (at & mu;M level) towards acid orange 7 (AO7) degradation was explored. Experimental results displayed that nearly 97.5% of AO7 could be removed within 15 min using 20 & mu;M Cu(II) and 0.4 mM SPC. Effects of Cu(II) concentration, SPC concentration, pH value and coexisting anions were investigated. Compared with conventional Fenton oxidation, which could only work under acidic pH con...

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