Multifunctional Ultrathin Ti3C2Tx MXene@CuCo2O4 /PE Separator for Ultra-High-Energy-Density and Large-Capacity Lithium-Sulfur Pouch Cells - 成果

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Multifunctional Ultrathin Ti₃C₂T_x MXene@CuCo₂O₄ /PE Separator for Ultra-High-Energy-Density and Large-Capacity Lithium-Sulfur Pouch Cells

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成果类型：

期刊论文

作者：

Huang, Zimo;Liang, Yuhao;Wu, Zhenzhen;Kong, Yang;Bai, Maohui;...

通讯作者：

Chen, Hao;Zhang, SQ;Bai, MH;Hong, B

作者机构：

[Liang, Yuhao; Huang, Zimo; Li, Meng; Zhang, Shanqing; Huang, Senchuan; Chen, Hao; Chen, H] Guangdong Univ Technol, Inst Sustainable Transformat, Sch Chem Engn & Light Ind, Guangzhou 510006, Peoples R China.

[Liang, Yuhao; Huang, Zimo; Li, Meng; Zhang, Shanqing; Huang, Senchuan; Chen, Hao; Chen, H] Jieyang Ctr, Guangdong Prov Lab Chem & Fine Chem Engn, Jieyang 515200, Peoples R China.

[Wu, Zhenzhen; Zhang, Shanqing] Griffith Univ, Ctr Catalysis & Clean Energy, Sch Environm & Sci, Gold Coast Campus, Gold Coast, Qld 4222, Australia.

[Kong, Yang] Shandong Univ, Inst Frontier & Interdisciplinary Sci, Sci Ctr Mat Creat & Energy Convers, Qingdao 266237, Peoples R China.

[Bai, Maohui] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410004, Peoples R China.

通讯机构：

[Bai, MH ; Hong, B ] C

[Chen, H; Zhang, SQ ] G

Guangdong Univ Technol, Inst Sustainable Transformat, Sch Chem Engn & Light Ind, Guangzhou 510006, Peoples R China.

Jieyang Ctr, Guangdong Prov Lab Chem & Fine Chem Engn, Jieyang 515200, Peoples R China.

Griffith Univ, Ctr Catalysis & Clean Energy, Sch Environm & Sci, Gold Coast Campus, Gold Coast, Qld 4222, Australia.

语种：

英文

关键词：

high-energy-density;lithium dendrites;lithium-sulfur batteries;multifunctional separator;polysulfides shuttling

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2025

卷：

期：

页码：

e2410318

DOI：

10.1002/adma.202410318

基金类别：

Postdoctoral Research Foundation of China; National Natural Science Foundation of China Research Fund for International Scientists [22250710135]; Innovative Leading Talents of The Double Thousand Plan of Jiangxi Province [jxsq2023102001]; Natural Science Foundation of Guangdong Province [2024A1515012077]; [GZC20230562]; [GZC20230564]

机构署名：

本校为通讯机构

院系归属：

材料科学与工程学院

摘要：

The shuttling of lithium polysulfides (LiPSs), sluggish reaction kinetics, and uncontrolled lithium deposition/stripping remain the main challenges in lithium-sulfur batteries (LSBs), which are aggravated under practical working conditions, i.e., high sulfur loading and lean electrolyte in large-capacity pouch cells. This study introduces a Ti(3)C(2)T(x) MXene@CuCo(2)O(4) (MCC) composite on a polyethylene (PE) separator to construct an ultrathin MXene@CuCo(2)O(4)/PE (MCCP) film. The MCCP functional separator can deliver superior LiPSs adsorptio...

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Multifunctional Ultrathin Ti₃C₂T_x MXene@CuCo₂O₄ /PE Separator for Ultra-High-Energy-Density and Large-Capacity Lithium-Sulfur Pouch Cells

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