Multifunctional Ultrathin Ti3C2Tx MXene@CuCo2O4 /PE Separator for Ultra-High-Energy-Density and Large-Capacity Lithium-Sulfur Pouch Cells

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成果类型：

期刊论文

作者：

Huang, Zimo;Liang, Yuhao;Wu, Zhenzhen;Kong, Yang;Bai, Maohui;...

通讯作者：

Chen, Hao;Zhang, SQ;Bai, MH;Hong, B

作者机构：

[Liang, Yuhao; Huang, Zimo; Li, Meng; Zhang, Shanqing; Huang, Senchuan; Chen, Hao; Chen, H] Guangdong Univ Technol, Inst Sustainable Transformat, Sch Chem Engn & Light Ind, Guangzhou 510006, Peoples R China.

[Liang, Yuhao; Huang, Zimo; Li, Meng; Zhang, Shanqing; Huang, Senchuan; Chen, Hao; Chen, H] Jieyang Ctr, Guangdong Prov Lab Chem & Fine Chem Engn, Jieyang 515200, Peoples R China.

[Wu, Zhenzhen; Zhang, Shanqing] Griffith Univ, Ctr Catalysis & Clean Energy, Sch Environm & Sci, Gold Coast Campus, Gold Coast, Qld 4222, Australia.

[Kong, Yang] Shandong Univ, Inst Frontier & Interdisciplinary Sci, Sci Ctr Mat Creat & Energy Convers, Qingdao 266237, Peoples R China.

[Bai, Maohui] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410004, Peoples R China.

通讯机构：

[Bai, MH ; Hong, B ] C

[Chen, H; Zhang, SQ ] G

Guangdong Univ Technol, Inst Sustainable Transformat, Sch Chem Engn & Light Ind, Guangzhou 510006, Peoples R China.

Jieyang Ctr, Guangdong Prov Lab Chem & Fine Chem Engn, Jieyang 515200, Peoples R China.

Griffith Univ, Ctr Catalysis & Clean Energy, Sch Environm & Sci, Gold Coast Campus, Gold Coast, Qld 4222, Australia.

语种：

英文

关键词：

high-energy-density;lithium dendrites;lithium-sulfur batteries;multifunctional separator;polysulfides shuttling

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2025

卷：

期：

页码：

e2410318

DOI：

10.1002/adma.202410318

基金类别：

National Natural Science Foundation of China Research Fund for International Scientists, (22250710135) Innovative Leading Talents of The Double Thousand Plan of Jiangxi Province, (jxsq2023102001) Postdoctoral Research Foundation of China, (GZC20230564, GZC20230562) Postdoctoral Research Foundation of China Natural Science Foundation of Guangdong Province, (2024A1515012077) Natural Science Foundation of Guangdong Province

机构署名：

本校为通讯机构

院系归属：

材料科学与工程学院

摘要：

The shuttling of lithium polysulfides (LiPSs), sluggish reaction kinetics, and uncontrolled lithium deposition/stripping remain the main challenges in lithium-sulfur batteries (LSBs), which are aggravated under practical working conditions, i.e., high sulfur loading and lean electrolyte in large-capacity pouch cells. This study introduces a Ti(3)C(2)T(x) MXene@CuCo(2)O(4) (MCC) composite on a polyethylene (PE) separator to construct an ultrathin MXene@CuCo(2)O(4)/PE (MCCP) film. The MCCP functional separator can deliver superior LiPSs adsorptio...

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Multifunctional Ultrathin Ti3C2Tx MXene@CuCo2O4 /PE Separator for Ultra-High-Energy-Density and Large-Capacity Lithium-Sulfur Pouch Cells

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