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Insight into the influence of environmental factors on selenite removal from desulfurization wastewater by NZVI@AC: An experimental and theoretical study

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成果类型:
期刊论文
作者:
Wang, Li;Li, Yu;Zou, Renjie;Sun, Ruize;Tian, Hong;...
通讯作者:
Luo, Guangqian;Yao, H
作者机构:
[Yao, Hong; Yao, H; Wang, Li; Luo, Guangqian; Luo, GQ; Zou, Renjie; Sun, Ruize] Huazhong Univ Sci & Technol, Sch Energy & Power Engn, State Key Lab Coal Combust, Wuhan 430074, Peoples R China.
[Li, Yu] Jiangsu Univ Sci & Technol, Sch Energy & Power, Zhenjiang 212100, Peoples R China.
[Tian, Hong] Changsha Univ Sci & Technol, Sch Energy & Power Engn, Changsha 410114, Peoples R China.
[Luo, Guangqian] Shenzhen Huazhong Univ Sci & Technol, Res Inst, Shenzhen 518000, Peoples R China.
通讯机构:
[Yao, H ; Luo, GQ] H
Huazhong Univ Sci & Technol, Sch Energy & Power Engn, State Key Lab Coal Combust, Wuhan 430074, Peoples R China.
语种:
英文
关键词:
Se(IV) removal;Adsorption;Density functional theory;pH value;Dissolved oxygen
期刊:
Journal of Water Process Engineering
ISSN:
2214-7144
年:
2024
卷:
57
页码:
104674
基金类别:
In order to determine the transformation process of high valence iron into zero valence iron at high temperatures, the TGA curves were obtained on a thermogravimetric analyzer at a heating rate of 20 °C·min−1. The effect of the preparation temperature (600, 800, and 1000 °C) on the reaction of carbon-reduced iron was analyzed (Fig. 1a, b, and c). The equilibrium composition diagrams at different temperatures were given in Fig. S1. The TGA and DTG results showed that there were various reaction
机构署名:
本校为其他机构
院系归属:
能源与动力工程学院
摘要:
Nano zero-valent iron (NZVI) technology has shown good potential for the treatment of selenium in wastewater. In this study, NZVI was loaded on activated carbon (AC) by carbothermal reduction method to synthesize highefficiency adsorbent (NZVI@AC). The agglomeration of NZVI was suppressed and its reactivity was improved. The optimum preparation temperature of NZVI@AC (600 degrees C) was determined by comparing its purity. Moreover, the synergistic effect between the active component (NZVI) and the support (AC) was investigated on the basis of the density functional theory method. The smaller H...

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