Engineering active heterojunction architecture with oxygenated-Co, Mo bimetallic sulfide heteronanosheet and graphene oxide for peroxymonosulfate activation

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作者信息关键词期刊信息基础信息归属信息摘要

成果类型：

期刊论文

作者：

Xie, Qianqian;Wang, Xuxu;Chen, Wenqian*;Lei, Chao;Huang, Binbin*

通讯作者：

Chen, Wenqian;Huang, Binbin

作者机构：

[Xie, Qianqian; Wang, Xuxu; Huang, Binbin] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Peoples R China.

[Xie, Qianqian; Wang, Xuxu; Huang, Binbin] Hunan Univ, Key Lab Environm Biol & Pollut Control, Minist Educ, Changsha 410082, Peoples R China.

[Chen, Wenqian] Natl Univ Singapore, Dept Pharm, S9,4 Sci Dr 2, Singapore 117544, Singapore.

[Lei, Chao] Changsha Univ Sci & Technol, Sch Hydraul Engn, Changsha 410114, Peoples R China.

通讯机构：

[Huang, Binbin] K

[Chen, Wenqian] D

Department of Pharmacy, National University of Singapore, S9, 4 Science Drive 2, 117544, Singapore. Electronic address: wen.

Key Laboratory of Environmental Biology and Pollution Control, Hunan University, Ministry of Education, Changsha 410082, PR China. Electronic address:

语种：

英文

关键词：

Activation mechanism;Advanced oxidation processes (AOPs);Co-Mo bimetal sulfide (CoMoS);Peroxymonosulfate;Water remediation

期刊：

Journal of Hazardous Materials

ISSN：

0304-3894

年：

2023

卷：

448

页码：

130852

DOI：

10.1016/j.jhazmat.2023.130852

基金类别：

CRediT authorship contribution statement Qianqian Xie: Methodology, Investigation. Xuxu Wang: Methodology, DFT calculation. Wenqain Chen: Conceptualization, Methodology, Software, Investigation, Data Curation, Writing – review & editing. Chao Lei: Conceptualization, Methodology, Software, Validation, Formal analysis, Investigation, Data curation, Writing – review & editing. Binbin Huang: Conceptualization, Methodology, Software, Validation, Formal analysis, Supervision, Project administration, acquisition, Writing – review &

机构署名：

本校为其他机构

院系归属：

水利工程学院

摘要：

Bimetallic sulfides have distinctive catalytic property in activating peroxymonosulfate (PMS) for water remediation. Polyoxometalates as potential precursors have rarely been reported for the catalytic degradation of refractory organic pollutants. Herein, a composite catalyst of Co-Mo bimetallic sulfides supported onto graphene oxide (O-CoMoS/GO) with a heterojunction architecture was synthesized through a hydrothermal strategy with polyoxometalates ((NH(4))(4)[Co(II)Mo(6)O(24)H(6)]·6H(2)O) as the precursor and applied in the PMS activation. T...

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Engineering active heterojunction architecture with oxygenated-Co, Mo bimetallic sulfide heteronanosheet and graphene oxide for peroxymonosulfate activation

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