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Research on the mechanism of interaction between styrene–butadiene–styrene (Sbs) and asphalt based on molecular vibration frequency

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成果类型:
期刊论文
作者:
Zeng, Yuqin;Liu, Qicheng*;Zeng, Qing;He, Yuhao;Xu, Zhenghong
通讯作者:
Liu, Qicheng
作者机构:
[Liu, Qicheng; Zeng, Yuqin; Zeng, Qing] Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha 410114, Peoples R China.
[Liu, Qicheng; Zeng, Yuqin; Zeng, Qing] Changsha Univ Sci & Technol, Hunan Prov Key Lab Flexible Elect Mat Genome Engn, Changsha 410114, Peoples R China.
[Xu, Zhenghong; He, Yuhao] Changsha Univ Sci & Technol, Coll Mat Sci & Engn, Changsha 410114, Peoples R China.
通讯机构:
[Liu, Qicheng] C
Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha 410114, Peoples R China.
Changsha Univ Sci & Technol, Hunan Prov Key Lab Flexible Elect Mat Genome Engn, Changsha 410114, Peoples R China.
语种:
英文
关键词:
Aromatization;Asphaltenes;Binding energy;Blending;Butadiene;Chemical bonds;Density functional theory;Fourier transform infrared spectroscopy;Molecular vibrations;Polybutadienes;Resins;Styrene;Component theories;Interaction strength;Peak intensity;Physical blending;SBS-modified asphalt;Vibration spectrum;Asphalt
期刊:
Materials
ISSN:
1996-1944
年:
2021
卷:
14
期:
2
页码:
1-14
基金类别:
Funding: The authors gratefully acknowledge financial support from the Natural Science Foundation of Hunan Province (2020jj4097), the Special Project for Innovative Province Construction in Hunan Province (2019GK5058), the Key Projects of Changsha Science and Technology Plan (kq1901102), and the Key Laboratory of Genetic Engineering for Flexible Electronic Materials of Hunan Province (2018TP1022).
机构署名:
本校为第一且通讯机构
院系归属:
物理与电子科学学院
材料科学与工程学院
摘要:
Based on the four-component theory of asphalt, molecular models of the saturate, aromatic, resin, and asphaltene were constructed, respectively. The styrene–butadiene–styrene (SBS) polymer was used as the modifier. Using density functional theory (DFT) to study the effect of SBS on the molecular vibration of each component of asphalt, the vibration spectrums and binding energy of the systems composed of SBS and each component molecule of asphalt were calculated. Prepared SBS modified asphalt and measured Fourier transform infrared spectroscop...

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