National Natural Science Foundation of China (NSFC) [12274470, 62273361]; Hunan Province for Distinguished Young Scholars [2022JJ10070]
机构署名：
本校为其他机构
院系归属：
物理与电子科学学院
摘要：
We theoretically explore the precise control of a molecular polariton by strongly coupling the lowest three rotational states of a single molecule with a single-mode cavity. We examine two distinct cavity resonance configurations: a fundamental frequency cavity (wc = 2B with the rotational constant B) resonating with the lowest two rotational states, and a second harmonic cavity (wc = 4B) coupling with the first and second excited rotational states. We propose two control schemes based on the two polariton configurations and derive the corresponding pulse-area theorems to achieve a theoretical...
